The Iterative Self-Consistent Reaction-Field Method: The Refractive Index of Pure Water

نویسندگان

  • KRISTIAN O. SYLVESTER-HVID
  • KURT V. MIKKELSEN
  • MARK A. RATNER
چکیده

We present different microscopic models for describing electromagnetic properties of condensed phases and the models involve iterative self-consistent procedures for calculating the properties. We report calculations of the frequency-dependent refractive index of pure water. We investigate the importance of the first solvation shell and nonequilibrium solvent configurations, and present a procedure for estimating appropriate cavity sizes. © 2010 Wiley Periodicals, Inc. Int J Quantum Chem 111: 904–913, 2011

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تاریخ انتشار 2010